Department of Chemistry

Organic Chemistry

Research Image

Research in organic chemistry at UNC Chapel Hill covers a broad range of subjects from natural products synthesis to the study of organic free-radicals with time-resolved EPR spectroscopy. Research is often interdisciplinary and involves science at the frontiers of polymer chemistry, inorganic chemistry, physical chemistry, materials science and bioorganic chemistry. With nine faculty members formally in the organic division and a number of faculty members from other divisions whose research involves organic chemistry, graduate students find they have a wide range of choices for their doctoral research.

 

Current Topics of Interest

  • Natural Products Synthesis
  • Asymmetric Catalysis
  • Bioorganic Chemistry
  • Dynamic Combinatorial Chemistry
  • Molecular Recognition
  • Physical Chemistry of Free Radicals
  • Drug Development
  • Drug Delivery
  • Nanomaterial Fabrication
  • Polymer Synthesis

 

Research Projects

Individual investigators are engaged in, among other things, the following general research areas:

Alexanian
Synthesis and Organometallic Catalysis

Brookhart
Mechanisms of Metal-Catalyzed Reactions

Crimmins
Total Synthesis of Biologically Active Natural Products

DeSimone
Drug Delivery, Nanomedicine, PRINT

Forbes
Spin Chemistry, Electron Donor-Acceptor Chemistry

Gagné
Transition Metal Catalysis, Dynamic Combinatorial Chemistry

Johnson
Synthetic Methods, Catalysis, Total Synthesis

Lawrence
Drug Development, Enzyme Inhibitors, Light-Activated Agents

Waters
Bioorganic Chemistry, Molecular Recognition

You
Organic Photovoltaics, Organic Spintronics

 

Representative Publications

Formal [4 + 2] Cycloaddition of Donor−Acceptor Cyclobutanes and Aldehydes: Stereoselective Access to Substituted Tetrahydropyrans. Andrew T. Parsons and Jeffrey S. Johnson. J. Am. Chem. Soc., 2009, 131 (40), pp 14202–14203.

Controlling Peptide Folding with Repulsive Interactions between Phosphorylated Amino Acids and Tryptophan. Alexander J. Riemen and Marcey L. Waters. J. Am. Chem. Soc., 2009, 131 (39), pp 14081–14087.

Acquisition of a Potent and Selective TC-PTP Inhibitor via a Stepwise Fluorophore-Tagged Combinatorial Synthesis and Screening Strategy. Sheng Zhang, Lan Chen, Yong Luo, Andrea Gunawan, David S. Lawrence and Zhong-Yin Zhang. J. Am. Chem. Soc., 2009, 131 (36), pp 13072–13079.

Asymmetric Synthesis of (+)-Polyanthellin A. Matthew J. Campbell and Jeffrey S. Johnson. J. Am. Chem. Soc., 2009, 131 (30), pp 10370–10371.

Radical Reactions with Double Memory of Chirality (2MOC) for the Enantiospecific Synthesis of Adjacent Stereogenic Quaternary Centers in Solution: Cleavage and Bonding Faster than Radical Rotation. Marino J. E. Resendiz, Farnosh Family, Kerrian Fuller, Luis M. Campos, Saeed I. Khan, Natalia V. Lebedeva, Malcolm D. E. Forbes and Miguel A. Garcia-Garibay. J. Am. Chem. Soc., 2009, 131 (24), pp 8425–8433.

Kinetics and mechanism of thermal decomposition of kynurenines and biomolecular conjugates: Ramifications for the modification of mammalian eye lens proteins. Lyudmila V. Kopylova, Olga A. Snytnikova, Elena I. Chernyak, Sergey V. Morozov, Malcolm D. E. Forbes, and Yuri P. Tsentalovich. Org. Biomol. Chem., 2009, 7, 2958-2966.

Illuminating the Chemistry of Life: Design, Synthesis, and Applications of . Lee, HM; Larson, DR; Lawrence, DS. ACS Chem. Biol., 2009, 4 (6), pp 409–427.

Time-Resolved EPR Investigation of Potential Model Systems for Acrylate Polymer Main Chain Radicals Based on Esters of Kemp's Tri-Acid. Natalia V. Lebedeva, Elena V. Gorelik, Damaris Magnus-Aryitey, Terence E. Hill and Malcolm D. E. Forbes. J. Phys. Chem. B, 2009, 113 (19), pp 6623–6629.

Diastereoselective Synthesis of Pentasubstituted Γ-Butyrolactones from Silyl Glyoxylates and Ketones through a Double Reformatsky Reaction. Stephen N. Greszler, Jeffrey S. Johnson. Angewandte Chemie International Edition, Volume 48, Issue 20, Pages 3689-3691.

Visual Snapshots of Intracellular Kinase Activity at the Onset of Mitosis. Zhaohua Dai, Natalya G. Dulyaninova, Sanjai Kumar, Anne R. Bresnick, and David S. Lawrence. Chemistry & Biology; Volume 14, Issue 11, 26 November 2007, Pages 1254-1260.